《Nitrogen Enables the Intensity Modulation of Charge Transfer and Spin Paramagnetism in Graphdiyne》 was written by Zhang, Mingjia; Guan, Zhaoyong; Yang, Ze; Hu, Xiuli; Wang, Xiaoxiong; Long, Yun-Ze; Huang, Changshui. Recommanded Product: 2,4,6-Trichloropyrimidine And the article was included in Chemistry of Materials in 2020. The article conveys some information:
The modulation of intrinsic properties, including magnetism in 2-dimensional materials, has attracted considerable interest as it expands device performance and allows for advanced flexible electronics. Herein, a facile way is developed to modulate the magnetic and elec. response of graphdiyne (GDY) by precise N doping. The introduced N exists only as specific pyridine N and can meet the relative change of 1:2:3 between different materials, which can be used as a switch-like property to manipulate charge transfer and spin. Among these, triazine-graphdiyne (TA-GDY) with the most N content achieves the highest saturation magnetization of up to 3.0 emu/g at 2 K. The accompanying moderate band gap and mobility of up to 7.56 cm2 V-1 s-1 endow it a broad application prospect. These results revealed that controllable N doping can modulate the phys. properties of C-based materials, thus providing a critical way to extend their application in future C electronics involving spin. The experimental part of the paper was very detailed, including the reaction process of 2,4,6-Trichloropyrimidine(cas: 3764-01-0Recommanded Product: 2,4,6-Trichloropyrimidine)
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Referemce:
Pyrimidine | C4H4N2 – PubChem,
Pyrimidine – Wikipedia